Surface physics course program

Surface thermodynamics. (Furio Ercolessi)

The Gibbs surface. Surface free energy and surface tension. Capillarity phenomena. Surface entropy. Anisotropy and surface stress. Kirkwood-Buff formula. Orientational dependence of surface free energy. Wulff construction and equilibrium shape. The equilibrium shape as a Gibbs free energy. Steps and vicinal surfaces. Faceting. Temperature dependence of equilibrium shape. Kinks. Step-step interactions. Pokrovsky-Talapov exponent. Roughening. Results of SOS (DG) and BCSOS models. Roughening of vicinal surfaces. Preroughening. Solid-liquid interfaces. Wetting and contact angles. Surface melting, non-melting, blocked melting. The effective interaction potential between SL and LV interfaces: short range forces and long-range forces. A Ginzburg-Landau theory of surface melting. Diffusion on a melted surface. Wetting of melt droplets on nonmelting surfaces. Non-melting-induced faceting. Halperin-Nelson-Young theory of 2D melting: hexatic phase, experimental observations.
Notation for crystal surfaces. A quick survey of experimental techniques: real space methods (HREM, FIM, STM/AFM), reciprocal space methods (LEED, He- and X-Ray scattering), indirect methods (LEIS/MEIS/HEIS, PhD, SEXAFS). Adsorption and chemisorption. Crystal growth: growth modes (FV,SK,VW). Capillary theory of nucleation. Epitaxy.

Metal surfaces. (Furio Ercolessi)

Glue models to describe atomic interactions in metals: failures of pairwise models, connection with tight-binding, parametrizations. Relaxation. Notations to describe surface superstructures. Contractive reconstructions. The triangular reconstruction of Au(100), Pt(100) and Ir(100): structure, microscopic origin, Frank and van der Merwe model and topological solitons, overlayer rotation, temperature behavior. Spontaneous formation of stress domains. The contractive reconstruction of Au(111) and Pt(111): structure, herringbone cell, temperature behavior. Magic vicinals. Faceting-driven reconstructions: Au(110), Pt(110) and Ir(110) missing row structures. The 1x2->1x1 decostruction of Au(110) and Pt(110): Ising universality class, disordered flat and rough phases. Alkali-induced reconstructions [K,Cs,Li,Na/Cu,Ni,Ag,Pd]. Displacive reconstructions. W(100) and Mo(100): Phase diagram, incommensurate phases, XY model with cubic anisotropy, effect of H and O. Liquid metal surfaces: structure and orientational order.

First-principles calculations of metal surfaces. Surface phonons. (Andrea Dal Corso)

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Furio Ercolessi
furio@sissa.it